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studies of current-induced precession in magnetic films. In various relations that exist among them. Here, we proceed
their pioneering work, Slonczewski4 and Berger5 used ana- phenomenologically and decompose the total number density
lytic model calculations to predict the critical current for the of conduction electrons into majority and minority contribu-
onset of precession in spin-valve structures with uniform but tions n⫽n ↑ ⫹n ↓ so that the current-induced deviations of
noncollinear magnetizations in the two ferromagnetic layers. these quantities from their equilibrium values are related by
Recent work shows that the seemingly different answers they
obtained are not inconsistent.11 Two global studies of preces- ␦ n⫽ ␦ n ↑ ⫹ ␦ n ↓ . 共1兲
sion and switching in single-domain spin valves12 and single-
domain particles13 supplement the Landau-Lifshitz-Gilbert In the drift-diffusion approximation, the particle current in
equation with the spin-transfer torque derived in Ref. 4. Ba- the nonmagnet is
zaliy et al.14 relaxed the assumption of uniform magnetiza-
tion and studied the effect of a legislated spin current flowing jNM⫽ 共 /e 兲 E⫺D“ ␦ n, 共2兲
from a nonmagnet into a semi-infinite ferromagnet. They where E is the electric field, is the conductivity, and D is
found that spontaneous excitation of spin waves occurs when the electron diffusion constant. We speak of spin accumula-
the current density is sufficiently large. Finally, we draw at- tion in the nonmagnet when the spin density
tention to a very recent application15 of magnetoelectronic
circuit theory16 to study current-induced precession in an ul- ប
trathin ferromagnetic film with uniform magnetization. For m⫽ 共 ␦ n ↑ ⫺ ␦ n ↓ 兲 m̂ 共3兲
unpolarized current densities above a critical value, the au- 2
thors predict that unstable spin-wave modes exist only for is different from zero. Notice that we use the particle current
nonzero wave vectors parallel to the interface. Our results and the spin density as variables rather than the charge cur-
confirm this prediction. rent and the magnetization.
The calculations presented in this paper combine phenom- A so-called spin-current density
enological constitutive equations for the electric current and
the spin current 共drift-diffusion equations兲 with a Landau- NM
Q ␣ ⫽⫺D“  m ␣ 共4兲
Lifshitz-Gilbert equation generalized to include spin-transfer
torque. The boundary conditions at each nonmagnet/ flows in the nonmagnet when the spin accumulation is not
ferromagnet interface are chosen so that relevant observables uniform in space. In Eq. 共4兲, the first index of Q ␣NM
,  labels the
reproduce the results of a Boltzmann equation treatment of ␣ th Cartesian component of the electron spin vector while
the same problem. Using experimental data to fix the param- the second index labels the  th Cartesian component of the
eters, we choose a value for the electric current density, and flow direction.
solve for the interface charge density 共chemical potential dis- In the ferromagnet, we make explicit use of the fact that
continuity兲, spin accumulation, and spin current assuming a there is no appreciable spin accumulation or spin current in
precessing magnetization with an amplitude and phase that the direction perpendicular to the magnetization.9,17 Accord-
depend on the running variable z in Fig. 1. The presumed ingly, ␦ m⫽(ប/2)( ␦ n ↑ ⫺ ␦ n ↓ ) is the spin accumulation so
precession is a legitimate mode of the system if the com-
puted spin-transfer torque balances the ferromagnetic ex- M⫽ 共 m s ⫹ ␦ m 兲 u 共5兲
change torque at each interface.14 The mode is unstable is the total spin density. Here, u is a unit vector, m s
共spontaneous excitation in the presence of a current兲 if the ⫽បM s /g B , and M s is the saturation magnetization. We
imaginary part of the mode frequency is negative. The mode adopt a two-current model18 so jFM⫽j↑ ⫹j↓ , where
is stable and uninteresting if Gilbert damping overwhelms
the effect of spin transfer. j↑ ⫽ 共 ↑ /e 兲 E⫺D ↑ “ ␦ n ↑ ,
The plan of this paper is as follows. In Sec. II, we set
down the basic definitions and equations of the theory. Sec- j↓ ⫽ 共 ↓ /e 兲 E⫺D ↓ “ ␦ n ↓ , 共6兲
tion III gives a qualitative picture of the origin of the preces-
sional instability. The boundary conditions for the transport using an obvious notation for the conductivity and diffusion
and magnetization equations are given in Sec. IV. Sections V constants of majority and minority spin electrons. Combin-
and VI present the details of the calculation for a single- ing all the above, the total particle current in the ferromagnet
interface geometry and a thin-film geometry, respectively. is
Section VII discusses our results. Section VIII examines the
effect of nonmagnetic leads using a reservoir geometry.15
↑⫹ ↓ D ↑ ⫹D ↓ D ↑ ⫺D ↓
jFM⫽ E⫺ “ ␦ n⫺ “ ␦ m. 共7兲
Section IX discusses some limitations of our model and sug- e 2 ប
gestions for future work. Section X is a summary. Appendix
A derives the effective exchange field for a bounded ferro- The corresponding spin current density in the ferromagnet
magnet. The transport boundary equations are derived in Ap- is
pendix B.
1
FM
Q ␣ ⫽ បu ␣ 共 j↑ ⫺j↓ 兲  . 共8兲
II. DEFINITIONS AND BASIC EQUATIONS 2
In an earlier paper,9 we defined the fundamental variables Consistent with our neglect of transverse spin accumulation
of spin transport quantum mechanically and described the in Eq. 共5兲, this formula presumes that the spin part of the
054408-2
PHENOMENOLOGICAL THEORY OF CURRENT-INDUCED . . . PHYSICAL REVIEW B 69, 054408 共2004兲
spin current in a ferromagnet is always parallel to the spin III. ORIGIN OF THE INSTABILITY
density. Then, using Eq. 共6兲, we get
Two characteristic features of the spin current Q ␣ under-
ប ↑⫺ ↓ ប D ↑ ⫺D ↓ lie the qualitative physics of current-induced precession.
FM
Q ␣ ⫽ u ␣E ⫺ u ␣“ ␦ n First, the structure of the spin-transfer torque in Eqs. 共11兲 and
2 e 2 2
共12兲 implies that the magnetization at the z⫽0 interface in
D ↑ ⫹D ↓ Fig. 1 feels a torque per unit area. It is
⫺ u ␣ “  ␦ m. 共9兲
冕
2 Nst ⑀
NM
⫽⫺ lim dz“•Q⫽ 共 QNM⫺QFM兲 •ẑ⯝Q⬜ ⬘ z , 共14兲
Textbooks show that the charge density inside a current- A ⑀ →0 ⫺⑀
carrying Ohmic conductor is zero 共except within a screening
distance of an interface or free surface兲. Therefore, we are where ⬜ ⬘ refers to the directions transverse to the ferromag-
justified to put ␦ n⫽0 in Eqs. 共2兲, 共7兲, and 共9兲. We will also netic magnetization (z ⬘ is the direction along the ferromag-
netic magnetization兲. The last line in Eq. 共14兲 is true because
fix the current to be j⫽ j 0 ẑ everywhere. Using this fact in Eq.
共7兲, we can eliminate E from Eq. 共9兲 and simplify the com- NM FM
Q z ⬘ z ⫽Q z ⬘ z 共15兲
ponents of the ferromagnetic spin current density that flow in
directions longitudinal 共z兲 and transverse (⬜) to the interface FM
and Q⬜ ⬘ z ⯝0 at the interface between a nonmagnet and a
normal. The result is ferromagnet due to spin filtering and other effects.4,5,9,19
The second bit of information we need is a linear kinetic
1
z ⫽ ប ␥ u ␣ j 0 ⫺D z u ␣ “ z ␦ m,
Q ␣FM p equation that relates the transverse spin current at the inter-
2 NM
face, Q⬜ ⬘ z , to the interfacial densities of our problem
共charge accumulation, spin accumulation in the nonmagnet,
⬜ ⫽⫺D⬜ u ␣ “⬜ ␦ m,
Q ␣FM 共10兲
and ferromagnetic spin accumulation兲. Of these, for a static
where ␥ p⫽( ↑ ⫺ ↓ )/( ↑ ⫹ ↓ ) is the degree of current po- magnetization only the spin accumulation m in Eq. 共3兲 has a
larization desired by the ferromagnetic bulk, D z ⫽(D ↑ ↓ transverse component. Therefore, it must be the case that
⫹D ↓ ↑ )/( ↑ ⫹ ↓ ) is an effective longitudinal spin diffu- NM
sion constant, and D⬜ ⫽ 21 (D ↑ ⫹D ↓ ) is an effective transverse Q⬜ ⬘ z ⫽bm⬜ ⬘ , 共16兲
spin-diffusion constant. where b is a constant. More detailed considerations 共see Ap-
The equation of motion for the spin density in the non-
pendix B兲 show that b⬎0.
magnet is a continuity equation for the spin accumulation.9
For simplicity, we will study 共in this section兲 a time-
Taking account of distributed spin-transfer torque, spin-flip
independent situation where electrons flow from a nonmag-
scattering, and torque from the external magnetic field, we
net into a ferromagnet with a small amplitude, frozen spin
find
wave at the interface. That is, in Eq. 共5兲, we let u⫽ẑ
m␣ ⫹u⬜ exp(iK•R), where R and K are two-dimensional vec-
ṁ ␣ ⫹“  Q ␣
NM
⫹ ␥ 关 m⫻Hext兴 ␣ ⫹ ⫽0, 共11兲 tors in the plane of the interface. This means that conduction
sf
electrons incident on the ferromagnet from the nonmagnet
where sf is the spin-flip scattering time in the nonmagnet see a static magnetization
and ␥ H⫽(g B /ប)B. The equation of motion for the spin
density in the ferromagnet is the Landau-Lifshitz-Gilbert M⫽M 兵 Re关 u⬜ e iK•R兴 ,Im关 u⬜ e iK•R兴 ,1其 . 共17兲
equation supplemented by a term to account for spin-transfer
torque as in Eq. 共11兲. Specifically, In the nonmagnet itself, Eqs. 共4兲 and 共11兲 with Hext⫽0
combine to give
u ␣␦ m
Ṁ ␣ ⫹“  Q ␣
FM
⫹ ␥ 关 M⫻Heff兴 ␣ ⫹ ⫽0, 共12兲 m␣
¯ sf Dⵜ 2 m ␣ ⫽ 共18兲
sf
where ¯ sf is the spin-flip scattering time in the ferromagnet. for the steady-state spin accumulation in the nonmagnet.
The effective field Heff accounts for the external field, ex- This is solved by
change, and damping,
m⫽ 兵 Re关 m⬜ 共 z 兲 e iK•R兴 ,Im关 m⬜ 共 z 兲 e iK•R兴 ,m z 共 z 兲 其 , 共19兲
0 l ex
2
␣
Heff⫽Hext⫹ ⵜ 2 M⫺ Ṁ. 共13兲 if
␥ms ␥ 兩 M兩
m z 共 z 兲 ⫽m z exp共 z/l sf兲 ,
Here, l ex⫽ 冑2A ex / 0 M s2 is the exchange length in a ferro-
magnet with spin stiffness A ex , 0 ⫽ ␥ M s , and ␣ is a phe- m⬜ 共 z 兲 ⫽m⬜ exp共 z 兲 共20兲
nomenological damping parameter. We ignore magnetostat-
ics, but for fields and magnetization perpendicular to the with 2
l sf ⫽D sf
and 2 2
l sf ⫽1⫹l sf2K 2 .
interface, its main effect is to shift the applied magnetic field We begin our analysis with the right side of the top panel
by an amount M s . in Fig. 2. This shows a spin pattern in the ferromagnet that is
054408-3
M. D. STILES, JIANG XIAO, AND A. ZANGWILL PHYSICAL REVIEW B 69, 054408 共2004兲
FIG. 3. 共a兲 Interfacial spin current and spin for current flow
from the nonmagnet into the ferromagnet. This diagram is the same
as Fig. 2共e兲. 共b兲 Same as 共a兲 except that the current flows from the
ferromagnet into the nonmagnet.
054408-4
PHENOMENOLOGICAL THEORY OF CURRENT-INDUCED . . . PHYSICAL REVIEW B 69, 054408 共2004兲
Finally, we remark that the presence of a second ‘‘polar- amplitude precessional motion around Hext⫽Hẑ. That is, we
izer’’ ferromagnetic film upstream in Fig. 2 tends to enhance
assume 共here and in all subsequent work兲 that u⫽ẑ⫹u⬜ with
the precessional instability. Even the K⫽0 mode can become
u⬜ Ⰶ1:
unstable as long as the magnetization of the polarizer is not
collinear with the magnetization of the ‘‘analyzer.’’ This is so j 0 ⫽ ␦ n 0 关 w 0 共 X ↑ ⫹X ↓ 兲兴 ⫹2ប ⫺1 m z 关 w 0 共 X ↑ ⫺X ↓ 兲兴
because, in that case, the electrons incident on the z⫽0 plane
carry a spin current with a nonzero component in a direction ⫺2ប ⫺1 ␦ m 关 X ↑ w ↑ ⫺X ↓ w ↓ 兴 ,
perpendicular to M. As a practical matter, this means that the
critical current for the onset of precession is lower when two NM
Q xz ⫽u x Q zz
NM
⫹w 0 共 m x ⫺u x m z 兲 ,
ferromagnets are present than for the case of a single ferro-
yz ⫽u y Q zz ⫹w 0 共 m y ⫺u y m z 兲 ,
Q NM
magnet studied by us. NM
0 l ex
2
where A FS is the area of the Fermi surface projected onto the
S
Hex ⫽ 关 ␦ 共 z 兲 ⫺ ␦ 共 z⫺t 兲兴 z M. 共21兲
␥ms interface. The constants w ↑ and w ↓ are defined similarly with
the densities of states per spin n ↑ / ↑ and n ↓ / ↓ . Fi-
This shows that a localized torque acts on each interface in nally,
Fig. 1共b兲. For the single-interface geometry, the ␦ (z⫺t) term
is absent. Spin-wave calculations for bounded 1⫺R
ferromagnets21 eliminate the surface torque produced by Eq. X ⫽ , 共25兲
4R
共21兲 by imposing the boundary condition z M⫽0 at each
interface. For our problem, the spin-transfer torque 共14兲 also where R↑ ⫽ 兩 R ↑ 兩 2 and R↓ ⫽ 兩 R ↓ 兩 2 are the squares of the ma-
acts at each interface. This dictates that we determine the jority and minority electron reflection amplitudes averaged
spin-wave modes by imposing a zero net torque requirement over the Fermi surface. The appearance of the interfacial
at each interface.14 The specific boundary condition is charge accumulation ␦ n 0 on the right side of Eq. 共23兲 is not
inconsistent with our earlier statement that ␦ n NM⫽ ␦ n FM
Nex⫹Nst⫽0. 共22兲 ⫽0 in the bulk. There is a resistance associated with the
interface whenever R ⫽0. The corresponding voltage drop
where Nex is the exchange torque density nex integrated over may be thought of as arising from a dipole layer of charge
an infinitesimally thin pillbox as in Eq. 共14兲.
difference ␦ n 0 localized at the interface.
A distribution of charge/spin current where the spins pre-
cess at a complex frequency ⫽ R⫹i I is a mode of the We note in closing that if u⬜ were zero (M储 ẑ), the second
system if Eq. 共11兲 is satisfied in nonmagnetic regions, Eq. and third boundary conditions in Eq. 共23兲 reduce to Eq. 共16兲.
共12兲 is satisfied in ferromagnetic regions, and Eq. 共22兲 is Appendix B demonstrates that the terms proportional to u⬜
satisfied at every interface. When I⬎0, the mode is stable in Eq. 共23兲 account for the fact that M is slightly tilted away
and uninteresting because its amplitude never grows large from the interface normal.
enough to be observed. True current-induced precession cor-
responds to modes with I⬍0. V. SINGLE INTERFACE GEOMETRY
Of course, the currents must also be consistent with the
We showed in Sec. III that spin-transfer torque can induce
spin-dependent scattering that occurs at the interface be-
a precessional instability. To discover if it actually does so
tween a magnet and a nonmagnet. Previously, two of the
requires a full solution of the coupled transport/
present authors10 addressed this issue by imposing scattering
magnetization dynamics equations with their boundary con-
boundary conditions on a 2⫻2 matrix Boltzmann equation
ditions. In particular, we need convenient formulas for the
and computing all observables from the semiclassical distri-
interfacial torques that enter Eq. 共22兲. For the single-interface
bution functions g ↑ (k,r) and g ↓ (k,r). In this paper, we ap- geometry of Fig. 1共a兲, a suitable precessional ansatz for the
ply boundary conditions to the observables directly in a man- magnetization in the nonmagnet is
ner that is consistent with this Boltzmann equation treatment.
We show in Appendix B that the boundary conditions m⫽ 兵 Re关 m⬜ 共 z 兲 ⌽ 兴 ,Im关 m⬜ 共 z 兲 ⌽ 兴 ,m z 共 z 兲 其 , 共26兲
obtained in this way take the form of a set of linear kinetic
i(K•R⫹ t)
equations which relate the interfacial currents to the interfa- where ⌽⫽e . The corresponding ansatz in the fer-
cial densities. Here, we quote a form that is valid for small romagnet is
054408-5
M. D. STILES, JIANG XIAO, AND A. ZANGWILL PHYSICAL REVIEW B 69, 054408 共2004兲
M 共 z 兲 ⫽m s⫹ ␦ m 共 z 兲 . 共29兲 Nex 0 l ex
2
0 l ex
2
⫽⫺ M⫻ z M⫽⫺i M 2 共 z 兲 u⬘⬜ 共39兲
A ms ms
A. Interfacial spin-transfer torque because
To find the spin-transfer torque, we substitute Eqs. 共26兲
and 共28兲 into the longitudinal component of the equations of ẑ⫻u⬜ ⫽iu⬜ 共40兲
motion 共11兲 and 共12兲. The solutions are 关cf. Eq. 共20兲兴
corresponds to a 90° rotation of the vector u⬜ . Since the
m z 共 z 兲 ⫽m z exp共 z/l sf兲 共30兲 function M (z) in Eq. 共29兲 is known at this point, the only
and unknown in Eq. 共39兲 is u⬜⬘ ⫽ z u⬜ (z) 兩 z⫽0 .
We determine u⬜⬘ numerically by integrating the trans-
␦ m 共 z 兲 ⫽ ␦ m exp共 ⫺z/ l̄ sf兲 共31兲 verse component of the Landau-Lifshitz-Gilbert equation
共12兲 inward from z⫽⬁ to z⫽0. The equation of interest is
2
with l̄ sf ⫽D z¯ sf . These are used in the longitudinal compo-
nent of Eqs. 共4兲 and 共10兲 to get the interfacial relations
NM
Q zz ⫽⫺ 共 D/l sf兲 m z ⫽Q zz 共32兲
0⫽ 兵 i ⫹ ␣ ⫺i ␥ H 其 u⬜ ⫹
1 1
M共z兲 2 再 冎
ប ␥ p j 0 ⫺D z M ⬘ 共 z 兲 u⬜⬘
0 M 共 z 兲 l ex
再 M ⬘共 z 兲
冎
2
and
⫹i u⬜⬙ ⫹2 u⬘ ⫺K 2 u⬜ . 共41兲
ms M共z兲 ⬜
⫽2
FM 1
Q zz ប ␥ j 0 ⫺ 共 D z / l̄ sf兲 ␦ m⫽Q zz .
p
共33兲
The previous two equations, together with the first and last The first term in brackets comes from the Ṁ ␣ , damping, and
共longitudinal兲 boundary conditions in Eq. 共23兲, determine the external field terms. The second term in brackets comes from
four interfacial quantities ␦ n 0 , m z , ␦ m, and Q zz in terms of the spin-transfer torque in the bulk of the ferromagnet due to
the spatial variation of the magnetization. The third term in
j 0 , ␥ p, D/l sf , D z / l̄ sf , X ↑ , X ↓ , w 0 , w ↑ , and w ↓ . In particu- brackets is the bulk exchange torque. On account of Eq. 共31兲,
lar, all four are proportional to j 0 , and thus change sign when
the current reverses as argued earlier. the spin-flip term u⬜ ␦ m/¯ sf in Eq. 共12兲 cancels a piece of the
spin-transfer torque. To derive Eq. 共41兲, we have used Eq.
Returning to Eq. 共26兲, we choose Hext⫽Hẑ, so the trans- 共40兲 repeatedly and exploited the identity
verse component of Eq. 共11兲 is solved by
where satisfies Very far from the interface, M (z)→m s and Eq. 共41兲 re-
duces to
2 2
l sf ⫽1⫹l sf2K 2 ⫹i sf共 ⫺ ␥ H 兲 共35兲
rather than the formulas quoted after Eq. 共20兲. Using Eq. 0⫽ 共 i ⫹ ␣ ⫺i ␥ H⫺i 0 K 2 l ex
2
兲 u⬜ ⫹ 21 ប ␥ p共 j 0 /m s兲 u⬜⬘
共34兲, the transverse component of Eq. 共4兲 yields
⫹i 0 l ex
2
u⬙⬜ . 共43兲
NM
Q⬜z ⫽⫺D m⬜ 共36兲
This equation is solved by u⬜ (z)⫽u⬜ exp(⫺p z) where
while the transverse boundary conditions in Eq. 共23兲 are (Re p⬎0),
NM
Q⬜z ⫺u⬜ Q zz
NM
⫽w 0 共 m⬜ ⫺u⬜ m z 兲 . 共37兲 ⍀ 1
pl ex⫽⫺i ⫾ 冑⫺⍀ 2 ⫺4 0 ⌬, 共44兲
From these, we can solve for the interfacial quantities NM
Q⬜z 20 20
and m⬜ . The spin-transfer torque follows straightforwardly
from Eq. 共14兲 when we follow Appendix B and express Q⬜ ⬘ z
NM and ⌬⫽ ⫺i ␣ ⫺ ␥ H⫺ 0 K 2 l ex
2
, where
in unprimed coordinates 共z-axis parallel to the interface nor-
mal兲 rather than primed coordinates (z ⬘ axis parallel to M): ប ␥ pj 0
⍀⫽ . 共45兲
2l exm s
Nst l sf⫺1
⫽Q⬜z
NM
⫺u⬜ Q zz
NM
⫽u⬜ ⌳ Q . 共38兲 This solution is used to start the inward integration of Eq.
A l sf⫹⌳ zz
共41兲. We note in passing that if ␣ ⫽K⫽0 and q⫽i p, Eq.
The constant ⌳⫽w 0 l sf /D. 共44兲 simplifies to
054408-6
PHENOMENOLOGICAL THEORY OF CURRENT-INDUCED . . . PHYSICAL REVIEW B 69, 054408 共2004兲
共 q 兲 ⫽ ␥ H⫹ 0 l ex
2 2
q ⫺⍀l exq. 共46兲 M 共 z 兲 ⫽m s⫹ ␦ m Lcsch共 t/ l̄ sf兲 sinh关共 t⫺z 兲 / l̄ sf兴
This is 共essentially兲 the dispersion relation derived by Baza- ⫹ ␦ m Rcsch共 t/ l̄ sf兲 sinh共 z/ l̄ sf兲 . 共50兲
liy and co-workers14 for bulk spin waves in the presence of a
specified spin current. An instability occurs ( goes nega- Up to an overall sign, the spin transfer and exchange
tive兲 when the current is large enough that ⍀ 2 ⬎4 0 ␥ H. If torques are still given by Eqs. 共38兲 and 共39兲. Therefore, at the
we take 0 H⫽1 T, this gives a charge current density J 0 right interface, we choose u⬜ arbitrarily and compute u⬜⬘ so
⫽ 兩 e 兩 j 0 ⬎10⫻109 A/cm2 , which is an order of magnitude that Eq. 共22兲 is satisfied at that interface. This provides the
larger than the interfacial instabilities we discuss below. initial condition for the integration of Eq. 共41兲 toward z
It is now straightforward to search for precession-type ⫽0. Then, the search through complex frequency space for
instabilities. For given values of current j 0 , external mag- solutions that satisfy Eq. 共22兲 at the left interface proceeds as
netic field H, and transverse wave vector K, we search described earlier. As initial guesses, we use the zero-current
through complex frequency ( ⫽ R⫹i I) space looking for frequencies of the spin-wave modes of the film,
modes. That is, situations where Eq. 共22兲 is satisfied using
Eq. 共38兲 for the interfacial spin-transfer torque and Eq. 共39兲 ␥ H⫹ 0 l ex
2
关共 n /t 兲 2 ⫹K 2 兴
n⫽ . 共51兲
for the interfacial exchange torque. If I⬍0, the mode is 1⫺i ␣
linearly unstable against precession. A suitable initial guess
is the zero-current surface spin-wave frequency VII. RESULTS AND DISCUSSION
␥ H⫹ 0 l ex
2
K2 The numerical results presented in this section are based
s⫽ . 共47兲 on converged solutions of the transport and magnetization
1⫺i ␣
equations using material parameters derived directly from
experiment or from first-principle electronic-structure calcu-
VI. THIN-FILM GEOMETRY lations 共Table I兲.
As in the preceding section, the search for current- A. Single-interface geometry
induced precessional instabilities in the thin-film geometry of
Fig. 1共b兲 begins by solving the longitudinal part of the prob- The top panel of Fig. 4 illustrates the regions of linear
lem. The spin accumulation decays exponentially into the instability as a function of applied charge current J 0 and
nonmagnetic leads so at the left (z⫽0) and right (z⫽t) in- wave vector K parallel to the interface for the single-
terfaces, we have the analog of Eq. 共32兲 for the interfacial interface geometry 共top panel of Fig. 1兲. An initial state of
spin currents: current-induced precession occurs inside each contour la-
beled by a choice of external magnetic field H. We empha-
size that every contour forms a closed loop in the J 0 -K
D sL D sR
L
Q zz ⫽⫺ L
m zL , R
Q zz ⫽⫺ R
m zR . 共48兲 plane. That is, for a fixed value of J 0 , the instability region is
l sf l sf bounded by a lower and an upper critical wave vector and,
for a fixed value of K, the instability region is bounded by a
The superscript on the diffusion constants and on the spin- lower and an upper critical current density. Note also that the
flip lengths allows us to assign different material properties instability occurs only for rather small values of external
to the leads and thus to the interfaces.15 magnetic field. We will see in the following subsection that
The z dependences of the spin accumulation and the spin thin films support precession for much larger values of H. In
current in the ferromagnetic film are linear combinations of addition, it appears that the upper critical field is very sensi-
exp(⫾z/l̄ sf). Straightforward algebra yields the interfacial re- tive to the parameters that describe the system. A systematic
lations exploration of parameter space is prohibitive, but we note
that the choices l sf⫽1000 nm and l̄ sf⫽15 nm give regions of
Dz instability for H⬎2 T.
L
Q zz ⫽ ␥ pj 0⫺ 关 ␦ m Lcoth共 t/ l̄ sf兲 ⫺ ␦ m Rcsch共 t/ l̄ sf兲兴 , The bottom panel of Fig. 4 is the same as the top panel
l̄ sf
except that we have replaced the full transverse Landau-
Lifshitz-Gilbert equation 共41兲 by
再 冎
Dz
R
Q zz ⫽ ␥ pj 0⫺ 关 ⫺ ␦ m Rcoth共 t/ l̄ sf兲 ⫹ ␦ m Lcsch共 t/ l̄ sf兲兴 . 1 1
l̄ sf 0⫽ 兵 i ⫹ ␣ ⫺i ␥ H 其 u⬜ ⫹ ប ␥ p j 0 ⫺D z M ⬘ 共 z 兲 u⬜⬘
共49兲 ms 2
The four equations in Eqs. 共48兲 and 共49兲, together with the
⫹i 0 l ex
2
兵 u⬜⬙ ⫺K 2 u⬜ 其 . 共52兲
two longitudinal boundary conditions in Eq. 共23兲 at each This approximation neglects the ferromagnetic spin accumu-
interface, determine the eight quantities ␦ n L0 , ␦ n R0 , m zL , m zR , lation ␦ m(z) in the exchange interaction and retains only its
␦ m R, ␦ m L, Q zz
L R
, and Q zz in terms of the physical parameters gradient variation in the bulk spin-transfer torque. Evidently,
of the model. Finally, because it is used in the integration of these omissions make no difference to the qualitative fea-
Eq. 共41兲, we record that tures of the diagram.
054408-7
M. D. STILES, JIANG XIAO, AND A. ZANGWILL PHYSICAL REVIEW B 69, 054408 共2004兲
(Cu) 6 n⍀ m 22
↑ 40.5 n⍀ m 22
↓ 109.5 n⍀ m 22
l sf(Cu) 450 nm 23
l̄ sf(Co) 59 nm 24
AR ↑ 0.117 f⍀ m2 22
AR ↓ 0.903 f⍀ m2 22
A FS 580 nm⫺2 25
n/ 6.23 eV⫺1 nm⫺3 26
n↑ /↑ 8.17 eV⫺1 nm⫺3 26
n↓ /↓ 31.6 eV⫺1 nm⫺3 26
A ex 2⫻10⫺11 J/m 27
Ms 14.46⫻105 A/m 28
␥ (Co) 1.9⫻1011 s⫺1 T⫺1 29
␥ (Cu) 1.75⫻1011 s⫺1 T⫺1 25
␣ 0.01 30
0⫽ 兵 i ⫹ ␣ ⫺i ␥ H 其 u⬜ ⫹
1 1
ms 2再 冎
ប ␥ p j 0 ⫺D z ␦ m 共 0 兲 / l̄ sf u⬜⬘
R⫽ 再 j 20
冋 冉 冊 冉 冊册
␥ ⬘ p⌳ ⬘
Q zz
⫹⌳ ⬘ 2
Q zz 2
⫹i 0 l ex
2
兵 u⬜⬙ ⫺K 2 u⬜ 其 . 共53兲 0 l ex
2
m s2 j0 j0
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PHENOMENOLOGICAL THEORY OF CURRENT-INDUCED . . . PHYSICAL REVIEW B 69, 054408 共2004兲
B. Thin-film geometry
We remarked at the end of Sec. III that the interfacial spin
torque associated with current flow from a ferromagnet to a
nonmagnet is opposite in direction to the interfacial spin
torque associated with current flow from a nonmagnet to a
ferromagnet. As pointed out by Polianski and Brouwer,15 this
implies that zero net spin torque acts on a uniformly magne-
tized film attached to identical leads at identical interfaces.
FIG. 5. Dependence on external magnetic field H of the critical
Those authors used leads of different lengths to break the
precession frequency crit divided by the Larmor frequency 共top
mirror symmetry of this geometry. We discuss that case in
panel兲, the critical parallel wave vector K crit 共middle panel兲, and the
critical current density J crit 共bottom panel兲 for the single-interface
more detail in the following section.
geometry of Fig. 1共a兲. In our calculations for a ferromagnetic film sandwiched
between two semi-infinite, nonmagnetic leads 共middle panel
of Fig. 1兲, the natural spatial variation of the magnetization
The second line in Eq. 共57兲 confirms our expectation of the spin-wave modes breaks the longitudinal symmetry.
about the behavior of the mode frequencies and thus ratio- Additional spatial variation arises because there is current-
nalizes the topology of Fig. 4. Moreover, this analytic for- induced mixing amongst the modes 共Fig. 6兲. As in the single-
mula for R agrees quantitatively with the real part of the interface problem, the spatial variation M (z) is essential for
mode frequencies we find from our numerical solution of the precession if we assume a symmetrical geometry where the
full equations of motion. Unfortunately, Eq. 共57兲 also pre- scattering properties of the two interfaces are identical. We
dicts I⬎0. That is, Eq. 共53兲 predicts only stable spin do this here, even though the formulas given in Sec. VI allow
waves. These modes are unstable in the full solution of Eq. for a more general, asymmetrical situation.
共52兲, but only barely so ( I is negative but very small in Figure 7 illustrates precessional instability diagrams for a
magnitude兲. In fact, the stability or instability of a given ferromagnetic film of thickness t⫽40 nm. For each value of
mode turns out to be an extremely sensitive function of the external magnetic field, the integer that labels each tear-drop-
phase of u⬜⬘ (0)/u⬜ (0) and the factor M ⬘ (z) in Eq. 共52兲. The shaped region indicates the mode that goes unstable in that
latter is determined by the ferromagnetic spin-flip length l̄ sf .
We conclude that variation of the magnetization with the
longitudinal variable z is an essential ingredient for instabil-
ity to occur in the single-interface geometry.
Figure 5 shows the calculated field dependence of the
critical frequency crit , the critical transverse wave vector
K crit , and the critical current density J crit , where precession
first occurs in the single-interface case. Consistent with Eq.
共57兲, all three are finite as H→0. Otherwise, crit and J crit
vary roughly linearly with field, as they do in experiments
performed on single films,7 until the instability shuts off for
large enough H. The order of magnitude of the critical cur-
rent (⬇109 A/cm2 ) is also consistent with the single-film
experiments 共and roughly ten times larger than the critical FIG. 7. Instability diagram for a t⫽40 nm ferromagnetic film in
current seen in the trilayer pillars studied in Ref. 1兲. Note, the geometry of Fig. 1共b兲 for three values of external magnetic field.
finally, that crit deviates systematically from the Larmor fre- The integers label the thin-film precessional mode that goes un-
quency ␥ H. stable in each region.
054408-9
M. D. STILES, JIANG XIAO, AND A. ZANGWILL PHYSICAL REVIEW B 69, 054408 共2004兲
054408-10
PHENOMENOLOGICAL THEORY OF CURRENT-INDUCED . . . PHYSICAL REVIEW B 69, 054408 共2004兲
054408-11
M. D. STILES, JIANG XIAO, AND A. ZANGWILL PHYSICAL REVIEW B 69, 054408 共2004兲
relatively better 共for tⰇl ex) as the lengths of the two leads mally activated magnetic reversal induced by a spin-
become more dissimilar. Qualitatively, this occurs because polarized current.31
there are two sources of net spin transfer torque in this prob-
lem: the longitudinal asymmetry of the leads and the longi- X. SUMMARY
tudinal asymmetry of the magnetization. If the first domi-
nates the second 共strong lead asymmetry兲, it does not really We have combined a drift-diffusion description of trans-
matter which mode goes unstable and the uniform magneti- port with a Landau-Lifshitz-Gilbert description of magneti-
zation approximation will be acceptable. If the second domi- zation dynamics to demonstrate that unpolarized current flow
nates the first 共weak lead asymmetry兲, the mode identity is from a nonmagnet into a ferromagnet can produce a
crucial and the approximate calculation fails badly. precession-type instability of the magnetization. Neglecting
magnetic anisotropy and magnetostatics, our numerical cal-
culations show 共for both single-interface and thin-film geom-
IX. LIMITATIONS AND FUTURE DIRECTIONS etries兲 that a linear instability occurs when both the current
In experiment, the large current densities required to pro- density and the excitation wave vector parallel to the inter-
duce current-induced precession are achieved using point- face are neither too small nor too large. The critical current
contact, nanowire, or nanopillar geometries where conductor density generally increases with increasing magnetic field
dimensions in the direction perpendicular to the current flow until the instability is quenched. Compared to the single-
are ‘‘necked-down’’ from micron-scale dimensions to hun- interface geometry, the film geometry supports a precessional
dred nanometer-scale dimensions. The reservoir geometry of instability over a much larger range of external magnetic
Fig. 1共c兲 is an approximate way to model this behavior field. In general, a particular spin-wave mode initiates the
within the context of a strictly one-dimensional calculation. instability when the mode just below it 共in energy兲 becomes
Nonetheless, it remains true that we have ignored the fact absolutely stable against current-induced precession.
that the current only acts over a small area. The small area is In a lead-film-lead geometry, it is necessary to break mir-
either a small part of a large film, or a small finite element. In ror symmetry to generate precession because equal and op-
both cases, we have ignored the behavior of the current at the posite spin transfer torques are generated at the two ends of
edges. the ferromagnetic film. In our model, the required symmetry
For a point-contact geometry, we have ignored how the breaking is provided by spin-wave modes of the film whose
current spreads into the film, how the variation in the mag- magnetization varies along the direction of current flow. If
netization decays into the film both laterally and in the inter- the magnetization is artificially constrained to be longitudi-
face direction, and how these interact. For a nanowire or nally uniform, asymmetry must be introduced in the length
nanopillar geometry, we have ignored the behavior of the or properties of the leads or in the scattering properties of the
current at the edges. Clearly, these three-dimensional effects two interfaces. When the spin-wave mode asymmetry gener-
will need to be considered if calculations of the sort pre- ates the spin-transfer torque, the critical current density first
sented here are ever to be truly predictive in the sense of decreases 共a quantum size effect兲 and then slowly increases
device design. 共as successive modes become stable against precession兲 as
Our calculations take no account of magnetostatics. The the film thickness increases. When interface or lead asymme-
necessary computations are a bit complex because the mag- try dominates the spin-transfer torque, the critical current is
netic self-energy is a nonlocal function of the spin density. It small 共compared to the mode-dominated regime兲 and slowly
is true that the dominant effect can be modeled as reducing increases due to increased damping as the film thickness in-
the applied field by 4 M s , but the known effects of magne- creases.
tostatics on spin-wave dispersion suggest the possibility of
other effects for the present problem. We also ignore any ACKNOWLEDGMENTS
intrinsic anisotropies present in real materials, such as mag-
One of us 共J.X.兲 acknowledges support from the National
netocrystalline anisotropy, anisotropic exchange, or aniso-
Science Foundation under Grant No. DMR-9820230. The
tropic damping. These anisotropies can be important for
authors thank Dr. Robert McMichael for essential help with
small applied fields.
the references.
More significantly, we have focused exclusively on the
initial, linear instability of a current-carrying nanomagnet to-
ward precession. In reality, nonlinear effects cut off the ex- APPENDIX A: EXCHANGE MAGNETIC FIELD
ponential growth of the mode amplitudes we find. This The total exchange energy of a semi-infinite ferromagnet
means that the final magnetic dynamical state may have little that extends from z⫽z L to z⫽z R is
in common with simple precession, particularly for magnets
冕 冕
whose size significantly exceeds an exchange length. To our
knowledge, little or nothing is known about spatially inho- A ex zR
E ex⫽ d 2R dz 共 ␣ M兲共 ␣ M兲 . 共A1兲
mogeneous magnetic states of this type in the present con- m s2 zL
text.
Finally, we have performed all of our calculations at zero The quantity m s occurs here because M denotes spin density
temperature. An extension to finite temperature clearly rather than magnetization. Focus on the ␣ ⫽z component and
would be interesting in light of recent experiments on ther- let M→M⫹ . This induces the variation
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PHENOMENOLOGICAL THEORY OF CURRENT-INDUCED . . . PHYSICAL REVIEW B 69, 054408 共2004兲
␦ E ex⫽
2A ex
m s2
冕 冕
d 2R
zR
zL
dz 共 z 兲 • 共 z M兲 . 共A2兲
j⫽ j ↑ ⫹ j ↓
⫽ 共 k ↑ ⫹k ↓ 兲 a 0 ␦ n NM⫺ 共 a ↑ k ↑ ⫹a ↓ k ↓ 兲 ␦ n FM
Integrating by parts gives 2 2
⫹ 共 k ⫺k 兲 a m ⫺ 共 a k ⫺a ↓ k ↓ 兲 ␦ m. 共B2兲
ប ↑ ↓ 0 z ប ↑ ↑
␦ E ex⫽
⫺2A ex
m s2
冕 冋冕 d 2R
zR
zL
dz • z2 M⫺ 关 • z M兲 兩 z R 册 z
L
The physical charge accumulation ␦ n 0 at the interface can
be partitioned arbitrarily between ␦ n NM and ␦ n FM. If we
共A3兲 choose ␦ n⫽ ␦ n NM and ␦ n FM⫽0, the boundary condition for
or the particle current becomes
j⫽ 共 k ↑ ⫹k ↓ 兲 a 0 ␦ n 0 ⫹2ប ⫺1 共 k ↑ ⫺k ↓ 兲 a 0 m z ⫺2ប ⫺1 共 a ↑ k ↑
␦ E ex⫽
⫺2A ex
m s2
冕 冕d 2R
zR
zL
dz • 兵 z2 M⫹ 共 z M兲关 ␦ 共 z⫺z L兲 ⫺a ↓ k ↓ 兲 ␦ m. 共B3兲
In exactly the same way, we derive the boundary condition
⫺ ␦ 共 z⫺z R兲兴 其 . 共A4兲 for the longitudinal spin current from
The exchange field H ex⫽⫺ ␥ ⫺1 ( ␦ E ex / ␦ M). Therefore, Q zz ⫽ j ↑ ⫺ j ↓
since ⬅ ␦ M,
1
2A ex ⫽ ប 共 k ↑ ⫺k ↓ 兲 a 0 ␦ n⫹ 共 k ↑ ⫹k ↓ 兲 a 0 m⫺ 共 a ↑ k ↑ ⫹a ↓ k ↓ 兲 ␦ m.
2
Hex⫽ 兵 z2 M⫹ 共 z M兲关 ␦ 共 z⫺z L兲 ⫺ ␦ 共 z⫺z R兲兴 其 .
␥ m s2 共B4兲
共A5兲
Equations 共B3兲 and 共B4兲 reproduce the first and last bound-
The ␣ ⫽x and ␣ ⫽y components of Eq. 共A1兲 do not generate ary conditions in Eq. 共23兲 if we use the Boltzmann equation
surface terms so Eq. 共A5兲 generalizes to treatment of the boundary conditions32 to make the choice
2A ex 2A ex A FS 1⫺R
Hex⫽ ⵜ 2 M⫹ 关 ␦ 共 z⫺z L兲 ⫺ ␦ 共 z⫺z R兲兴 z M. k ⫽ . 共B5兲
␥ms 2
␥ms 2 共 2 兲 3 ប 4R
共A6兲
We stated the boundary condition for the transverse spin
current in Sec. III, leaving a constant of proportionality b
APPENDIX B: TRANSPORT BOUNDARY CONDITIONS unspecified in Eq. 共16兲. As above, we choose this constant
for consistency with the Boltzmann equation treatment.32
The interfacial boundary conditions 共23兲 for the drift-
The result is
diffusion equations 共2兲, 共4兲, 共7兲, and 共9兲 can be derived most
convincingly by averaging the boundary conditions for the A FS
semiclassical distribution functions g ↑ (k,r) and g ↓ (k,r) NM
Q⬜z ⫽ a 0 m⬜ , 共B6兲
used in a Boltzmann equation treatment of spin transport.32 A 共 2 兲3ប
simpler alternative is to proceed phenomenologically and
where A FS is the area of the Fermi surface projected onto the
write kinetic equations that connect the currents to the den-
interface. The reflection coefficients in Eq. 共B5兲 do not ap-
sities. Temporarily, we assume that the ferromagnetic mag-
pear in Eq. 共B6兲 despite the fact that spins can rotate into the
netization M⫽M u is parallel to the interface normal, i.e., transverse direction upon quantum-mechanical reflection or
parallel to the z axis. transmission at an interface. This is so because the rotation
In linear approximation, the longitudinal particle current effect disappears after Fermi-surface averaging.9
that flows through the interface for each spin type is Tserkovnyak and co-workers33 discuss another contribu-
NM
tion to Q ␣ due to ‘‘spin pumping’’ from an adjacent ferro-
1
↑ ⫺ ↑ 兲 ⫽ k ↑ 共 a 0 ␦ n ↑ ⫺a ↑ ␦ n ↑ 兲 ,
j ↑ ⫽k ↑ 共 NM FM NM FM magnet. When the magnetization is time harmonic with fre-
2 quency , the time derivative of the magnetization can have
a component that is transverse to the magnetization and there
1 is an additional term in Eq. 共B6兲
↓ ⫺ ↓ 兲 ⫽ k ↓ 共 a 0 ␦ n ↓ ⫺a ↓ ␦ n ↓ 兲 . 共B1兲
j ↓ ⫽k ↓ 共 NM FM NM FM
2
A FS A FS ប
Here, k ↑ and k ↓ are kinetic coefficients, NM
↑ , ↓ , ↑ ,
NM FM NM
Q⬜z ⫽ a 0 m⬜ ⫹ u⬜ . 共B7兲
共2兲 ប
3
共 2 兲3 2
and FM
↓ are electrochemical potentials, and a 0 , a ↑ , and a ↓
are twice the inverse density of states per spin at the Fermi For our choice of parameters, this new term is numerically
level for electrons in the nonmagnet and for majority and much smaller than the other term except for high frequencies
minority electrons in the ferromagnet, respectively. Using and low currents. Nevertheless, we have retained it for all the
Eq. 共B1兲, the same algebra that led from 共6兲 to 共7兲 now yields calculations presented here.
054408-13
M. D. STILES, JIANG XIAO, AND A. ZANGWILL PHYSICAL REVIEW B 69, 054408 共2004兲
example,
NM A FS
Q⬜ ⬘ z ⫽ a 0 m⬜ ⬘ , 共B8兲
共 2 兲3ប
replaces Eq. 共B6兲 as the boundary condition for the trans-
verse spin current. However, because the direction of u⬜ in
Fig. 12 varies along the interface when the excitation wave
vector K⫽0, it behooves us to evaluate Eq. 共B8兲 using the
original, interface-referenced coordinates xyz.
The transformation law between the xyz and x ⬘ y ⬘ z ⬘ co-
ordinate systems 共Fig. 12兲 simplifies considerably when u⬜
Ⰶ1, as is the case for our problem. Then,
A x⬘ ⫽A x ⫺u⬜ A z ,
for any vector A that lies close to the z axis, This rule shows
As a final step, we must take explicit account of the fact that Eq. 共B8兲 is indeed identical to the transverse boundary
that M is tilted slightly away from the interface normal ẑ. conditions stated in Eq. 共23兲. It also shows that the longitu-
This is not difficult if we define a new coordinate system dinal boundary conditions stated above are unaffected by the
x ⬘ y ⬘ z ⬘ where ẑ⬘ points along M 共Fig. 12兲. In that case, for fact that u⬜ ⫽0.
1
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The first term on the right side of Eq. 共10兲 shows that Q zz FM
is
8
S.I. Kiselev, J.C. Sankey, I.N. Krivorotov, N.C. Emley, R.J. positive deep in the bulk where ␦ m⫽0. The diffusive correction
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PHENOMENOLOGICAL THEORY OF CURRENT-INDUCED . . . PHYSICAL REVIEW B 69, 054408 共2004兲
24
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